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1. Sorption-based atmospheric water generation (SAWG) is a promising strategy to alleviate the drinkable water scarcity of arid regions.

2. A composite sorbent@biomimetic fibrous membrane (PPy-COF@Trilayer-LiCl) with hierarchically porous structure has been developed, which exhibits outstanding water uptake performance and fast water release capacity.

3. A wearable SAWG device has been established as a proof-of-concept demonstration, which can operate 10 sorption–desorption cycles per day in the outdoor condition and produce a high yield of clean water reaching up to 3.91 kg m−2 day−1.

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